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I sorted everything according to seasons and episodes:
Season 3:
3A:
3×01 The Heart of the Truest Believer:
– Peter Pan – Villains.
3×02 Lost Girl:
– The Lost Girl – Heroes.
3×03 Quite a Common Fairy:
– Tinkerbell and Regina – Heroes.
– Present Tense – Heroes.
3×04 Nasty Habits:
– The Pied Piper – Villains.
3×05 Good Form:
– Sky Sailing – Heroes.
3×06 Ariel:
– Ariel – Heroes.
3×07 Dark Hollow:
– Wendy Darling – Heroes.
3×09 Save Henry:
– Return To Storybrooke – Heroes.
3×11 Going Home:
– The Price For Regina – Heroes.
– Unhappy Ending – Heroes.
3B:
3×12 New York City Serenade:
– Almost Married A Monkey – Villains.
– The Wicked Witch – Villains.
3×14 The Tower:
– The Emma That Never Was – Heroes.
– The Witch and the Dagger – Villains.
– Rapunzel Returns – Heroes.
3×15 Quiet Minds:
– Lumiere – Villains.
– The Lion Tattoo – Heroes.
– A True Sacrifice – Heroes.
3×16 It’s Not Easy Being Green:
– A Hero’s Funeral – Heroes.
– The Wizard – Villains.
3×17 The Jolly Roger:
– Black Beard – Villains.
3×19 A Curious Thing:
– Glinda The Good Witch – Heroes.
3×21 Snow Drift:
– Emma and Elsa (the first half) – Heroes.
– Waltzing Emma – Heroes.
3×22 There’s No Place Like Home:
– Wedding in the Woods – Heroes.
– Bringing Bad – Villains.
Season 4 (counting by abc):
4A:
4×01 A Tale of Two Sisters:
– Anna and Elsa – Heroes.
– The Hat Box – Villains.
4×02 White Out:
– Bo Peep Battle – Villains.
– Emma and Elsa (the second half) – Heroes.
4×03 Rocky Road:
– The Knave (originally from Wonderland) – Heroes.
4×04 The Apprentice:
– The Dark One’s Apprentice – Villains.
4×05 Breaking Glass:
– What The Snow Queen Wants – Villains.
4×06 Family Business:
– Oaken’s – Heroes.
4×07 The Snow Queen:
– Kite Flying – Heroes.
4×09 Smash the Mirror, pt 2:
– Emma’s Magic – Heroes.
(I Actually haven’t found the full version, but some parts of the tracks were played seperately during 4×03, 4×07, 4×08, 4×09. I actually suspect that they were originally intended to use it in the scene at end where Emma is with her family and does fireworks with her magic. Play it there, it fits, If someone finds the scene where the full track plays, let me know).
4×10 Fall:
– The Snow Queen’s Spell – Villains.
– Shattered Heroes – Heroes. (Unused, confirmed that it was intended for this episode by Mark Isham).
4×11 Shattered Sight:
– Ingrid’s End – Villains.
4×12 Heroes and Villains:
– Queens of Darkness – Villains.
4B:
4×13 Darkness at the Edge of Town:
– Chernabog Problems – Villains.
4×14 Unforgiven:
– Maleficent – Villains.
4×16 Poor Unfortunate Soul:
– Ursula – Villains.
4×17 Best Laid Plans:
– Transferring Darkness – Villains.
– The Author – Villains.
4×18 Heart of Gold:
– Hood Heroics – Heroes.
– The Most Vile Villain – Villains.
4×19 Sympathy for the De Vil:
– Cruella De Vil – Villains.
– Cruella’s Sewing Project – Villains..
4×23 Operation Mongoose, pt 2:
– Emma Swan, The Dark One – Villains.
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